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化学气相沉积英文相关介绍

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2021-02-02 17:27
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2021年2月2日发(作者:烦)


A number of forms of CVD are in wide use and are frequently referenced


in


the


literature.


These


processes


differ


in


the


means


by


which


chemical


reactions are initiated (e.g., activation process) and process


conditions.


Classified by operating pressure:


o



Atmospheric pressure CVD


(APCVD)



CVD processes at


atmospheric pressure.


o



Low-pressure


CVD



(LPCVD)




CVD


processes


at


subatmospheric


pressures.


[1]


Reduced pressures tend to reduce unwanted


gas-phase reactions and improve film uniformity across the


wafer.


Most


modern


CVD


processes


are


either


LPCVD


or


UHVCVD.


o



Ultrahigh


vacuum


CVD



(UHVCVD)




CVD


processes


at


a


very


low


pressure, typically below 10


?


6



Pa


(~10


?


8



torr


). Note that in


other fields, a lower division between high and


ultra-high


vacuum


is common, often 10


?


7


Pa.


?



Classified by physical characteristics of vapor:


o



Aerosol assisted CVD


(AACVD)



A CVD process in which the


precursors are transported to the substrate by means of a


liquid/gas aerosol, which can be generated ultrasonically.


This technique is suitable for use with non-volatile


precursors.


o



Direct


liquid


injection


CVD



(DLICVD)




A


CVD


process


in


which


the


precursors


are


in


liquid


form


(liquid


or


solid


dissolved


in a convenient solvent). Liquid solutions are injected in


a vaporization chamber towards injectors (typically car


injectors).


Then


the


precursor


vapors


are


transported


to


the


substrate as in classical CVD process. This technique is


suitable for use on liquid or solid precursors. High growth


rates can be reached using this technique.


?



Plasma methods (see also


Plasma processing


):


o



Microwave plasma-assisted CVD


(MPCVD)


o



Plasma-Enhanced CVD


(PECVD)



CVD processes that utilize


plasma



to


enhance


chemical


reaction


rates


of


the


precursors.


[2]



PECVD processing allows deposition at lower temperatures,


which


is


often


critical


in


the


manufacture


of


semiconductors.


o



Remote plasma- enhanced CVD


(RPECVD)



Similar to PECVD


except


that


the


wafer


substrate


is


not


directly


in


the


plasma


discharge region. Removing the wafer from the plasma region


allows processing temperatures down to room temperature.


?



Atomic


layer


CVD



(


ALCVD


)




Deposits


successive


layers


of


different


substances


to


produce


layered,


crystalline



films.


See


Atomic


layer


epitaxy


.


?



?



Combustion Chemical Vapor Deposition


(CCVD)



nGimat's


proprietary Combustion Chemical Vapor Deposition process is an


open- atmosphere, flame-based technique for depositing


high-quality thin films and nanomaterials.


Hot wire CVD


(HWCVD)



also known as catalytic CVD (Cat-CVD) or


hot filament CVD (HFCVD). Uses a hot filament to chemically


decompose the source gases.


[3]



Metalorganic chemical vapor deposition


(MOCVD)



CVD processes


based on


metalorganic


precursors.


Hybrid Physical-Chemical Vapor Deposition


(HPCVD)



Vapor


deposition processes that involve both chemical decomposition of


precursor gas and


vaporization


of a solid source.


Rapid thermal CVD


(RTCVD)



CVD processes that use heating lamps


or


other


methods


to


rapidly


heat


the


wafer


substrate.


Heating


only


the substrate rather than the gas or chamber walls helps reduce


unwanted gas phase reactions that can lead to


particle


formation.


Vapor phase epitaxy


(VPE)


?



?



?



?



?



Uses


Integrated circuits


Various


CVD


processes


are


used


for


integrated


circuits



(ICs).


Particular


materials are deposited best under particular conditions.


Polysilicon


Polycrystalline silicon is deposited from


silane


(SiH


4


), using the


following reaction:


SiH


4



→ Si + 2 H


2



This reaction is usually performed in LPCVD systems, with either pure


silane feedstock, or a solution of silane with 70



80%


nitrogen


.


Temperatures between 600 and


650 °C and p


ressures between 25 and 150


Pa


yield


a


growth


rate


between


10


and


20


nm



per


minute.


An


alternative


process


uses


a


hydrogen


-based


solution.


The


hydrogen


reduces


the


growth


rate,


but


the temperature is raised to 850 or even 1050 °C to compensate.



Polysilicon


may


be


grown


directly


with


doping,


if


gases


such


as


phosphine


,


arsine


or


diborane


are added to the CVD chamber. Diborane increases the


growth rate, but arsine and phosphine decrease it.


Silicon dioxide


Silicon dioxide (usually called simply


industry)


may


be


deposited


by


several


different


processes.


Common


source


gases include


silane


and


oxygen


,


dichlorosilane


(SiCl

< br>2


H


2


) and


nitrous


oxide



(N


2


O),


or


tetraethylorthosilicate



(TEOS;


Si(OC


2


H


5


)


4


).


The


reactions


are as follows


[


citation needed


]


:


SiH


4


+ O


2



→ SiO


2


+ 2 H


2



SiCl


2


H


2


+ 2 N


2


O → SiO


2


+ 2 N


2


+ 2 HCl


Si(OC< /p>


2


H


5


)


4



→ SiO


2


+ byproducts


The


choice


of


source


gas


depends


on


the


thermal


stability


of


the


substrate;


for


instance,


aluminium



is


sensitive


to


high


temperature.


Silane


deposits


between


300


and


500


°C,


dichlorosilane


at


around


900


°C,


and


TEOS


between


650 and 750 °C, resulting in a layer of


low- temperature oxide


(LTO).


However, silane produces a lower- quality oxide than the other methods


(lower


dielectric


strength


,


for


instance),


and


it


deposits


non


conformally


.


Any of these reactions may be used in LPCVD, but the silane reaction is


also done in APCVD. CVD oxide invariably has lower quality than


thermal


oxide


, but thermal oxidation can only be used in the earliest stages of


IC manufacturing.


Oxide


may


also


be


grown


with


impurities


(


alloying



or



doping

< br>


This


may


have two purposes. During further process steps that occur at high


temperature, the impurities may


diffuse


from the oxide into adjacent


layers (most notably silicon) and dope them. Oxides containing 5



15%


impurities


by


mass


are


often


used


for


this


purpose.


In


addition,


silicon


dioxide alloyed with


phosphorus pentoxide


(


smooth out uneven surfaces. P-glass softens and reflows at temperatures


above 1000 °C. This process requires a phosphorus concentra


tion of at


least 6%, but concentrations above 8% can corrode aluminium. Phosphorus


is deposited from phosphine gas and oxygen:


4 PH


3


+ 5 O


2



→ 2 P


2


O


5


+ 6 H


2



Glasses



containing


both


boron


and


phosphorus


(borophosphosilicate


glass,


BPSG) undergo viscous flow at lower temperatures; around 850 °C is


achievable


with


glasses


containing


around


5


weight %


of


both


constituents,


but


stability


in


air


can


be


difficult


to


achieve.


Phosphorus


oxide


in


high


concentrations


interacts


with


ambient


moisture


to


produce


phosphoric


acid.


Crystals of BPO


4


can also precipitate from the flowing glass on cooling;


these crystals are not readily etched in the standard reactive plasmas


used


to


pattern


oxides,


and


will


result


in


circuit


defects


in


integrated


circuit manufacturing.

-


-


-


-


-


-


-


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